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Entropy? Never heard of it.
(lemmy.dbzer0.com)
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Why wouldn't the device include or feed a compressor to liquidize the CO2? It takes just a little over 5 atm of pressure which is trivial.
You also need to sustain 5 atm, with no leaks for years. Where is it being stored, and who's paying for the maintenance? All it would take would be a bit of civil unrest, or corruption, and the work could be undone in mass.