So many great answers already, but one I don't think I've seen mentioned yet is the soundtrack for Bastion
It's nice to see so many different awnsers, gaming has just so many good soundtracks.
Personally, I love the soundtrack of the original Xenoblade Chronicles. "Engage the Enemy" really hits during the cutscene it plays.
Another recomendation is Xenoblade Chronicles 3's "Words that never reached you"
Awesome for the Amiga
Final fantasy 6 Chrono trigger Street fighter 2 Street fighter v Super Mario Bros 3 Mega Man 2 Undertale And this is really unfair but Def Jam fight for New York
Super Mario Galaxy has an amazing soundtrack!
Def hollow knight, I think it captures the essence of a long decaying kingdom perfectly.
MW2: Mercenaries was pretty awesome.
Other ones that come to mind are Crazy Taxi and Tony Hawk's Pro Skater.
Team Fortress 2 OST
I love soundtracks from Splatoon, all series. Especially Chip Damage/Blitz it! is my favourite.
90% of the Sonic Frontiers "Cyberspace" tracks are S tier. The best soundtrack in recent memory.
Total Annihilation
There is a reason Touhou has two fandoms, one for its games and the other for its music. The music alone saved it from being another Oregon Trail and eventually got it its own anime.
IDK if it's best of all time but the soundtrack to Guardians Crusade, a jrpg for kids on the PS1, is pretty up there and waaaaaaayyyyyy better than it has any right to be.
I am personally in love with Far Cry 5's soundtrack.
Right now I'm going to have to go with a tie between Brok and Graff from Brok the Investigator and the legacy soundtrack piece After The Flames by Josh Woodward from SuperTuxKart.
Okami has a truly beautiful soundtrack, my favourites are the 'The Sun Rises' and The Eight Dog Warriors Theme'. Also Calamari Inkantation from Splatoon is fantastic.
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